Browsing by Author "Pagano, Fiammetta"
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Item Open Access Data supporting 'Two-dimensional perovskite functionalized fiber-type heterostructured scintillators'(Cranfield University, 2023-02-22 12:04) Rogers, Edith; Danang Birowosuto, Muhammad; Maddalena, Francesco; Dujardin, Christophe; Pagano, Fiammetta; Kratochwil, Nicolaus; Auffray, Etiennette; george Krause, Philip; Bizarri, GregoryData used to produce the article "Two-dimensional perovskite functionalized fibre-type heterostructured scintillators" Data used to create the 2D histograms of charge (fig 2) and the CTR plots (fig 3)Item Open Access Fast emitting nanocomposites for high-resolution ToF-PET imaging based on multicomponent scintillators(Wiley, 2024-02-28) Orfano, Matteo; Pagano, Fiammetta; Mattei, Ilaria; Cova, Francesca; Secchi, Valeria; Bracco, Silvia; Rogers, Edith; Barbieri, Luca; Lorenzi, Roberto; Bizarri, Gregory; Auffray, Etiennette; Monguzzi, AngeloTime-of-Flight Positron Emission Tomography (ToF-PET) is a medical imaging technique, based on the detection of two back-to-back γ-photons generated from radiotracers injected into the body. Its limit is the ability of employed scintillation detectors to discriminate in time the arrival of γ-pairs, that is, the coincidence time resolution (CTR). A CTR < 50 ps will enable fast imaging with ultralow radiotracer dose. Monolithic materials do not have simultaneously the required high light output and fast emission characteristics, thus the concept of scintillating heterostructure is proposed, where the device is made of a dense scintillator coupled to a fast-emitting light material. Here a composite polymeric scintillator loaded with hafnium oxide nanoparticles is presented. This enhanced by +300% its scintillation yield, by surpassing commercial plastic scintillators. The nanocomposite is coupled to bismuth germanate oxide (BGO) realizing a multilayer metascintillator. The energy sharing between its components is observed, which activates the nanocomposite's fast emission enabling a net CTR improvement of 25% with respect to monolithic BGO. These results demonstrate that a controlled loading with dense nanomaterials is an excellent strategy to enhance the performance of polymeric scintillators for their use in advanced radiation detection and imaging technologies.Item Open Access Two-dimensional perovskite functionalized fiber-type heterostructured scintillators(AIP Publishing, 2023-02-21) Rogers, Edith; Birowosuto, Muhammad Danang; Maddalena, Francesco; Dujardin, Christophe; Pagano, Fiammetta; Kratochwil, Nicolaus; Auffray, Etiennette; Krause, Philip George; Bizarri, GregoryA fiber-type heterostructured scintillator based on bismuth germanate (Bi4Ge3O12) functionalized with the 2D-perovskite butylammonium lead bromide ((BA)2PbBr4) has been fabricated, and its scintillation performance analyzed toward its use for fast timing applications such as time-of-flight Positron Emission Tomography. The pixel shows energy sharing between the matrix and filler component, confirming that the two components are in synergy.